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アクセス権	open access
URI	https://hdl.handle.net/2115/82004
タイトル	Iridium(III) Catalysts with an Amide-Pendant Cyclopentadienyl Ligand : Double Aromatic Homologation Reactions of Benzamides by Fourfold C-H Activation
著者	Tomita, Eiki ; Yamada, Kodai ; Shibata, Yu ; Tanaka, Ken ; Kojima, Masahiro ; Yoshino, Tatsuhiko ; Matsunaga, Shigeki
著者名 Tomita, Eiki
著者名 Yamada, Kodai
著者名 Shibata, Yu
著者名 Tanaka, Ken
e-Rad_Researcher 90824714 著者名 Kojima, Masahiro
e-Rad_Researcher 50756179 著者名 Yoshino, Tatsuhiko
e-Rad_Researcher 50334339 著者名 Matsunaga, Shigeki
言語	英語
キーワード	anthracenes
	aromatic homologation
	C-H activation
	cyclopentadienyl ligand
	iridium
発行日	2020-06-22
出版者	Wiley-Blackwell
収録物名	Angewandte chemie-international edition
巻(号)	59(26)
ページ	10474-10478
抄録	The synthesis, characterization, and catalytic performance of iridium(III) catalysts that bear an amide-pendant cyclopentadienyl ligand ([(CpIrI2)-Ir-A](2)) is reported. These [(CpIrI2)-Ir-A](2)catalysts were obtained from the complexation of a Cp(A)ligand precursor with [Ir(cod)OAc](2)followed by oxidation. Double aromatic homologation reactions of benzamides with alkynes by fourfold C-H activation proceeded in good to high yield with these [(CpIrI2)-Ir-A](2)catalysts, demonstrating their superior catalytic performance in this challenging transformation.
資源タイプ	学術雑誌論文
出版タイプ	Accepted Manuscript
権利情報	This is the peer reviewed version of the following article: Tomita, Eiki et al. Iridium(III) Catalysts with an Amide-Pendant Cyclopentadienyl Ligand: Double Aromatic Homologation Reactions of Benzamides by Fourfold C-H Activation. Angewandte chemie-international Edition, 2020,59,10474-10478. which has been published in final form at https://doi.org/10.1002/anie.202003009. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions.
PISSN	1433-7851
関連情報 (isVersionOf)	出版社版DOI https://doi.org/10.1002/anie.202003009

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