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アクセス権	open access
URI	https://hdl.handle.net/2115/97976
タイトル	Electrochemical N2O Reduction Reaction Catalyzed by a Multinuclear Copper Complex of 1,2,4-Triazole
著者	Ma, Zhengwei ; Kato, Masaru ; Watanabe, Takeshi ; Yagi, Ichizo
著者名 Ma, Zhengwei
e-Rad_Researcher 70709633 著者名 Kato, Masaru
e-Rad_Researcher 00750382 著者名 Watanabe, Takeshi
e-Rad_Researcher 40292776 著者名 Yagi, Ichizo
言語	英語
キーワード	N2O reduction
	electrocatalysis
	denitrification
発行日	2025-08-05
出版者	Oxford University Press
収録物名	Chemistry Letters
巻(号)	54(8)
ページ	upaf149
抄録	A trinuclear copper complex of 1,2,4-triazole supported on a carbon black efficiently catalyzes the electrochemical N2O reduction reaction (e-N2ORR) in alkaline media, achieving 100% Faradaic efficiency at -0.2 V vs. RHE and a turnover frequency up to 267 h-1 at -0.6 V vs. RHE. In situ X-ray absorption spectroscopy reveals that a Cu(0) species produced from the Cu(II) complex under electrochemical conditions is responsible for the high e-N2ORR activity and selectivity, offering a cost-effective strategy for efficient greenhouse gas mitigation.
資源タイプ	学術雑誌論文
出版タイプ	Accepted Manuscript
権利情報	This is a pre-copyedited, author-produced version of an article accepted for publication in Chemistry Letters following peer review. The version of record Zhengwei Ma, Masaru Kato, Takeshi Watanabe, Ichizo Yagi: Electrochemical N2O Reduction Reaction Catalyzed by a Multinuclear Copper Complex of 1,2,4-Triazole. Chemistry Letters, 5 August 2025: upaf149 is available online at: https://doi.org/10.1093/chemle/upaf149.
EISSN	1348-0715
関連情報 (isVersionOf)	出版社版DOI https://doi.org/10.1093/chemle/upaf149

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