open access

https://hdl.handle.net/2115/94250

Nonlinear frequency-asymmetric optical response in chiral systems

英語

2025-01-15

American Physical Society (APS)

Physical Review B

111(3)

035130

We report our theoretical results on the emergence of a nonlinear frequency-asymmetric optical response characteristic of chiral crystal systems with neither spatial inversion symmetry nor mirror symmetry. Based on the group theoretical analysis, we show that the chirality-related second-order nonlinear optical response occurs for two different input frequencies when the low-energy model Hamiltonian includes a time-reversal-even pseudoscalar quantity, i.e., the electric toroidal monopole. We demonstrate its emergence by investigating a fundamental microscopic model with the chiral-type antisymmetric spin-orbit interaction on a simple cubic lattice. By analyzing the behavior of nonlinear optical conductivity based on the Kubo formula, we find that the response is largely enhanced when one of the frequencies is set to 0 and the other is set to a resonant frequency. We also discuss the relaxation time dependence of the response.

学術雑誌論文

Accepted Manuscript

©[2025] American Physical Society

2469-9950