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Levels, potential sources and human health risk of polycyclic aromatic hydrocarbons (PAHs) in particulate matter (PM10) in Kumasi, Ghana
Title: | Levels, potential sources and human health risk of polycyclic aromatic hydrocarbons (PAHs) in particulate matter (PM10) in Kumasi, Ghana |
Authors: | Bortey-Sam, Nesta Browse this author | Ikenaka, Yoshinori Browse this author →KAKEN DB | Akoto, Osei Browse this author | Nakayama, Shouta M. M. Browse this author →KAKEN DB | Yohannes, Yared Beyene Browse this author | Baidoo, Elvis Browse this author | Mizukawa, Hazuki Browse this author →KAKEN DB | Ishizuka, Mayumi Browse this author →KAKEN DB |
Keywords: | Airborne particulate | PAHs | Kumasi | BaP toxic equivalent | Incremental lifetime cancer risk | Chemical mass balance |
Issue Date: | Jul-2015 |
Publisher: | Springer |
Journal Title: | Environmental Science and Pollution Research |
Volume: | 22 |
Issue: | 13 |
Start Page: | 9658 |
End Page: | 9667 |
Publisher DOI: | 10.1007/s11356-014-4022-1 |
PMID: | 25616380 |
Abstract: | Airborne particulate samples were collected on quartz filters to determine the concentrations, sources and health risks of polycyclic aromatic hydrocarbons (PAHs) in air in Kumasi, Ghana. A total of 32 air samples were collected in Kwame Nkrumah University of Science and Technology (KNUST) campus (pristine site) and city centre (CC). Samples were extracted with 1:2 v/v acetone:hexane mixture prior to GC-MS analyses. The sum of concentrations of 17 PAHs in air ranged from 0.51 to 16 (KNUST) and 19-38 ng/m3 (CC). The concentration of benzo[a]pyrene, BaP, ranged from below detection limit to 0.08 ng/m3 (KNUST) and 1.6 to 5.6 ng/m3 (CC). Chemical mass balance model showed that PAHs in air in Kumasi were mainly from fuel combustion. The total BaP equivalent concentration (BaPeq) in CC was 18 times higher compared to KNUST; based on the European Legislation and Swedish and UK Standards for BaP in air, CC could be classified as highly polluted. Estimated carcinogenicity of PAHs in terms of BaPeq indicated that BaP was the principal PAH contributor in CC (70 %). Health risk to adults and children associated with PAH inhalation was assessed by taking into account the lifetime average daily dose and corresponding incremental lifetime cancer risk (ILCR). The ILCR was within the acceptable range (10-6 to 10-4), indicating low health risk to residents. |
Rights: | The final publication is available at Springer via http://dx.doi.org/10.1007/s11356-014-4022-1 |
Type: | article (author version) |
URI: | http://hdl.handle.net/2115/62334 |
Appears in Collections: | 獣医学院・獣医学研究院 (Graduate School of Veterinary Medicine / Faculty of Veterinary Medicine) > 雑誌発表論文等 (Peer-reviewed Journal Articles, etc)
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Submitter: 石塚 真由美
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