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Thickness Optimization toward High-Performance Bottom-Gated Transparent Tin Dioxide Thin-Film Transistors

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Please use this identifier to cite or link to this item:http://hdl.handle.net/2115/83072

Title: Thickness Optimization toward High-Performance Bottom-Gated Transparent Tin Dioxide Thin-Film Transistors
Authors: Liang, Dou-Dou Browse this author
Chen, Binjie Browse this author
Cho, Hai Jun Browse this author
Ohta, Hiromichi Browse this author →KAKEN DB
Keywords: effective channel thickness
amorphous SnO2
transparent thin-film transistor
electric-field thermopower modulation
depletion layer
bottom-gated
Issue Date: 27-Oct-2020
Publisher: American Chemical Society
Journal Title: ACS Applied Electronic Materials
Volume: 2
Issue: 10
Start Page: 3454
End Page: 3458
Publisher DOI: 10.1021/acsaelm.0c00711
Abstract: Nowadays, transparent amorphous oxide semiconductor (TAOS)-based transparent thin-film transistors (TTFTs) are utilized as the backplane of organic light-emitting diode (OLED) displays. Among many TAOSs examined to date, amorphous (a-)SnO2 is one of the most promising candidates owing to its environmental compatibility, e.g., indium-free. Although several SnO2-based TFTs have been demonstrated so far, the reported characteristics are ambiguous, e.g., extremely high electron mobility (>100 cm(2) V-1 s(-1)) and behaviors far different from those of currently used a-InGaZnO4 -based TFTs. Here, we show high-performance bottom-gated a-SnO2-based TTFTs. First, we systematically investigated the electron transport properties and the band gap of SnO2 films with various thicknesses. Then, we optimized the SnO2 thickness by analyzing the operation mechanism of the TTFTs using an electric-field thermopower modulation technique. We found that the optimal SnO2 thickness is 4.2 nm for high-performance TTFTs (highest on-to-off current ratio (similar to 10(5)) and high mobility (similar to 20 cm(2) V-1 s(-1))). The present results would be essential to develop a-SnO2-based TTFTs in commercial applications.
Rights: This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Applied Electronic Materials, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://pubs.acs.org/doi/10.1021/acsaelm.0c00711 .
Type: article (author version)
URI: http://hdl.handle.net/2115/83072
Appears in Collections:電子科学研究所 (Research Institute for Electronic Science) > 雑誌発表論文等 (Peer-reviewed Journal Articles, etc)

Submitter: 太田 裕道

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