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Catalytic Methylation of Benzene over Pt/MoOx/TiO2 and Zeolite Catalyst Using CO2 and H-2

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Title: Catalytic Methylation of Benzene over Pt/MoOx/TiO2 and Zeolite Catalyst Using CO2 and H-2
Authors: Ting, Kah Wei Browse this author
Imbe, Takuto Browse this author
Kamakura, Haruka Browse this author
Maeno, Zen Browse this author →KAKEN DB
Siddiki, S. M. A. Hakim Browse this author
Matsushita, Koichi Browse this author
Shimizu, Ken-ichi Browse this author →KAKEN DB
Toyao, Takashi Browse this author →KAKEN DB
Keywords: CO2 hydrogenation
One-pot synthesis
Issue Date: Feb-2022
Publisher: 日本化学会(Chemical Society of Japan)
Journal Title: Chemistry letters
Volume: 51
Issue: 2
Start Page: 149
End Page: 152
Publisher DOI: 10.1246/cl.210664
Abstract: Catalytic methylation of benzene using CO2/H-2 was investigated using various combinations of supported metal catalysts and zeolites in a batch reactor. After a thorough catalyst screening process, the combination of Pt(3)/MoOx(30)/TiO2 and H-MOR (SiO2/Al2O3 = 90) was the most efficient, achieving up to 39% benzene-based yield and 27% CO2-based yield, without promoting the dearomatization of benzene, under the reaction conditions employed in this study (1 MPa CO2, 5 MPa H-2, 1 mmol of benzene, 240 degrees C, 12 h).
Type: article
Appears in Collections:触媒科学研究所 (Institute for Catalysis) > 雑誌発表論文等 (Peer-reviewed Journal Articles, etc)

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