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Liquid-Cell Transmission Electron Microscopy Observation of Two-Step Collapse Dynamics of Silicon Nanopillars on Evaporation of Propan-2-ol: Implications for Semiconductor Integration Density
| Title: | Liquid-Cell Transmission Electron Microscopy Observation of Two-Step Collapse Dynamics of Silicon Nanopillars on Evaporation of Propan-2-ol: Implications for Semiconductor Integration Density |
| Authors: | Sasaki, Yuta Browse this author | | Yamazaki, Tomoya Browse this author | | Kimura, Yuki Browse this author →KAKEN DB |
| Keywords: | capillary interactions | | collapse dynamics | | nanostructures | | in situ observation | | LC-TEM | | semiconductors |
| Issue Date: | 22-Jun-2022 |
| Publisher: | American Chemical Society |
| Journal Title: | ACS Applied Nano Materials |
| Volume: | 5 |
| Issue: | 7 |
| Start Page: | 9495 |
| End Page: | 9502 |
| Publisher DOI: | 10.1021/acsanm.2c01744 |
| Abstract: | Miniaturization of semiconductor devices has made structures more fragile, leading to potential collapses due to capillary forces during drying after wet cleaning. This has hampered the integration of transistors according to Moore's law. We have developed a method for preparing nanopillars in a liquid cell and have successfully observed their collapse by means of a crosssectional view in transmission electron microscopy. The dynamics of collapse as a result of capillary interactions involve two steps. First, the nanopillars collapse due to an imbalance in capillary forces caused by a difference in liquid levels at the gas-liquid interface. Second, a liquid pool formed between nanopillars maintains the collapsed state of the nanopillars through surface tension. The nanopillars recover on reimmersion in the liquid after the collapse. This method is effective, and is expected to contribute to the continued development of miniaturization and three-dimensionality of semiconductors. |
| Rights: | This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Applied Nano Materials, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://pubs.acs.org/articlesonrequest/AOR-5QHW6R8XTUHSUDH3DF6X. |
| Type: | article (author version) |
| URI: | http://hdl.handle.net/2115/90025 |
| Appears in Collections: | 低温科学研究所 (Institute of Low Temperature Science) > 雑誌発表論文等 (Peer-reviewed Journal Articles, etc)
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Submitter: 木村 勇気
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