Enantioselective Intramolecular C-H Amidation of Sulfamate Esters Catalyzed by Chiral Dirhodium(II) Carboxylates


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Please use this identifier to cite or link to this item:http://hdl.handle.net/2115/26429

Title:	Enantioselective Intramolecular C-H Amidation of Sulfamate Esters Catalyzed by Chiral Dirhodium(II) Carboxylates
Authors:	Yamawaki, Minoru Browse this author
	Kitagaki, Shinji Browse this author
	Anada, Masahiro Browse this author →KAKEN DB
	Hashimoto, Shunichi Browse this author →KAKEN DB
Issue Date:	1-Dec-2006
Publisher:	The Japan Institute of Heterocyclic Chemistry
Journal Title:	Heterocycles - An International Journal for Reviews and Communications in Heterocyclic Chemistry
Volume:	69
Issue:	1
Start Page:	527
End Page:	537
Abstract:	The chiral dirhodium(II) carboxylate-catalyzed enantioselective intramolecular C-H amidation reaction of sulfamate esters via in situ generated iminoiodinanes is described. The use of dirhodium(II) tetrakis[N-tetrafluorophthaloyl-(S)-tert-leucinate], Rh2(S-TFPTTL)4, as a catalyst and PhI(OAc)2 as an oxidant provides cyclic sulfamidates in up to 48% ee.
Type:	article (author version)
URI:	http://hdl.handle.net/2115/26429
Appears in Collections:	薬学研究院 (Faculty of Pharmaceutical Sciences) > 雑誌発表論文等 (Peer-reviewed Journal Articles, etc)

Submitter: 穴田仁洋

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