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Pincer-Type Phosphorus Compounds with Boryl-Pendant and Application in Catalytic H-2 Generation from Ammonia-Borane: A Theoretical Study

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Title: Pincer-Type Phosphorus Compounds with Boryl-Pendant and Application in Catalytic H-2 Generation from Ammonia-Borane: A Theoretical Study
Authors: Yang, Deshuai Browse this author
Bao, Panqing Browse this author
Yang, Zhen Browse this author
Chen, Zhaoxu Browse this author
Sakaki, Shigeyoshi Browse this author
Maeda, Satoshi Browse this author →KAKEN DB
Zeng, Guixiang Browse this author
Keywords: ammonia borane
theoretical study
dehydrogenation
pincer-type phosphorus
phosphorus-boryl cooperation
Issue Date: 3-Sep-2021
Publisher: Wiley-Blackwell
Journal Title: ChemCatChem
Volume: 13
Issue: 18
Start Page: 3925
End Page: 3929
Publisher DOI: 10.1002/cctc.202100661
Abstract: Metal-free catalysts composed of heavy main group element(s) have been limited. Herein, a theoretical study unveils that pincer-type phosphorus compound bearing a boryl-pendant is good catalyst for H-2 generation from ammonia borane through phosphorus-boryl (P-B) cooperation function. Pincer-type phosphorus compound without boryl-pendant is not active for this reaction, indicating the important role of the P-B cooperation function.
Type: article
URI: http://hdl.handle.net/2115/82595
Appears in Collections:理学院・理学研究院 (Graduate School of Science / Faculty of Science) > 雑誌発表論文等 (Peer-reviewed Journal Articles, etc)

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