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Solid-State C-N Cross-Coupling Reactions with Carbazoles as Nitrogen Nucleophiles Using Mechanochemistry

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Please use this identifier to cite or link to this item:http://hdl.handle.net/2115/87723

Title: Solid-State C-N Cross-Coupling Reactions with Carbazoles as Nitrogen Nucleophiles Using Mechanochemistry
Authors: Kubota, Koji Browse this author
Endo, Tsubura Browse this author
Uesugi, Minami Browse this author
Hayashi, Yuta Browse this author
Ito, Hajime Browse this author →KAKEN DB
Keywords: ball milling
carbazole
cross-coupling
mechanochemistry
solid-state reaction
Issue Date: 21-Jan-2022
Publisher: Wiley-Blackwell
Journal Title: ChemSusChem
Volume: 15
Issue: 2
Start Page: e202102132
Publisher DOI: 10.1002/cssc.202102132
Abstract: The palladium-catalyzed solid-state C-N cross-coupling of carbazoles with aryl halides via a high-temperature ball-milling technique has been reported. This reaction allowed simple, fast, and efficient synthesis of N-arylcarbazole derivatives in good to excellent yields without the use of large amounts of organic solvents in air. Importantly, the developed solid-state coupling approach enabled the cross-coupling of poorly soluble aryl halides with large polyaromatic structures that are barely reactive under conventional solution-based conditions.
Rights: This is the peer reviewed version of the following article: K. Kubota, T. Endo, M. Uesugi, Y. Hayashi, H. Ito, ChemSusChem 2022, 15, e202102132, which has been published in final form at https://doi.org/10.1002/cssc.202102132. This article may be used for non-commercial purposes in accordance with Wiley Terms and Conditions for Use of Self-Archived Versions. This article may not be enhanced, enriched or otherwise transformed into a derivative work, without express permission from Wiley or by statutory rights under applicable legislation. Copyright notices must not be removed, obscured or modified. The article must be linked to Wiley’s version of record on Wiley Online Library and any embedding, framing or otherwise making available the article or pages thereof by third parties from platforms, services and websites other than Wiley Online Library must be prohibited.
Type: article (author version)
URI: http://hdl.handle.net/2115/87723
Appears in Collections:工学院・工学研究院 (Graduate School of Engineering / Faculty of Engineering) > 雑誌発表論文等 (Peer-reviewed Journal Articles, etc)

Submitter: 久保田 浩司

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